Metal-Free Synthesis of N-Aryl Amides using Organocatalytic Ring-Opening Aminolysis of Lactones

doi:10.1002/cssc.201700415

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RECERCAT Home > Centres de Recerca de Catalunya (CERCA) > Institut Català d'Investigació Química (ICIQ) > Papers > View document

Use this identifier to quote or link this document: http://hdl.handle.net/2072/356181

dc.contributor.author	Guo, Wusheng
dc.contributor.author	Gómez, José Enrique
dc.contributor.author	Martínez-Rodríguez, Luis
dc.contributor.author	Bandeira, Nuno A. G.
dc.contributor.author	Bo, Carles
dc.contributor.author	Kleij, Arjan W.
dc.date.accessioned	2019-05-23T09:16:18Z
dc.date.available	2019-05-23T09:16:18Z
dc.date.issued	2017-05-09
dc.identifier.uri	http://hdl.handle.net/2072/356181
dc.format.extent	1969 p.
dc.language.iso	eng
dc.rights	L'accés als continguts d'aquest document queda condicionat a l'acceptació de les condicions d'ús establertes per la següent llicència Creative Commons:http://creativecommons.org/licenses/by-nc-nd/4.0/
dc.source	RECERCAT (Dipòsit de la Recerca de Catalunya)
dc.subject.other	54
dc.title	Metal-Free Synthesis of N-Aryl Amides using Organocatalytic Ring-Opening Aminolysis of Lactones
dc.type	info:eu-repo/semantics/article
dc.type	info:eu-repo/semantics/acceptedVersion
dc.embargo.terms	12 mesos
dc.identifier.doi	10.1002/cssc.201700415
dc.rights.accessLevel	info:eu-repo/semantics/openAccess
dc.description.abstract	Catalytic ring-opening of bio-sourced non-strained lactones with aromatic amines can offer a straightforward, 100% atom- economical and sustainable pathway towards relevant N-aryl amide scaffolds. We herein report the first general, metal-free and highly efficient N-aryl amide formation from poorly reactive aromatic amines and non-strained lactones under mild operating conditions using an organic bicyclic guanidine catalyst. This protocol has great application potential as exemplified by the formal syntheses of drug relevant molecules.

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