Nickel-Catalyzed Carboxylation of Benzylic C−N Bonds with CO2

doi:https://dx.doi.org/10.1002/anie.201600697

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RECERCAT Home > Centres de Recerca de Catalunya (CERCA) > Institut Català d'Investigació Química (ICIQ) > Papers > View document

Use this identifier to quote or link this document: http://hdl.handle.net/2072/226211

dc.contributor.author	Moragas, Toni
dc.contributor.author	Gaydou, Morgane
dc.contributor.author	Martin, Ruben
dc.date.accessioned	2018-01-15T16:03:24Z
dc.date.accessioned	2018-02-15T10:29:01Z
dc.date.available	2018-01-15T16:03:24Z
dc.date.available	2018-02-15T10:29:01Z
dc.date.issued	2016
dc.identifier.uri	http://hdl.handle.net/2072/226211
dc.identifier.uri	http://hdl.handle.net/2072/305934
dc.language.iso	eng
dc.publisher	Wiley
dc.relation	ICIQ foundation v the European Research Council
dc.relation	MINECO
dc.relation	Severo Ochoa Excellence Accreditation
dc.relation	European Union
dc.relation	European Research Council (ERC-277883)
dc.relation	MINECO (CTQ2012-34054) severo ochoa SEV-2013-0319
dc.relation.ispartof	Angew. Chem. Int.
dc.rights	© 1999 - 2016 John Wiley & Sons, Inc.
dc.subject.other	Nickel
dc.subject.other	C–N activation
dc.subject.other	Reductive coupling
dc.subject.other	Carboxylation
dc.subject.other	Catalysis
dc.title	Nickel-Catalyzed Carboxylation of Benzylic C−N Bonds with CO2
dc.type	info:eu-repo/semantics/article
dc.relation.projectID	info:eu-repo/grantAgreement/ERC/FP7/277883
dc.relation.projectID	CTQ2012-34054
dc.relation.projectID	SEV-2013-0319)
dc.identifier.doi	https://dx.doi.org/10.1002/anie.201600697
dc.rights.accessLevel	info:eu-repo/semantics/openAccess
dc.description.abstract	A user-friendly Ni-catalyzed reductive carboxylation of benzylic C−N bonds with CO₂ is described. This procedure outperforms state-of-the-art techniques for the carboxylation of benzyl electrophiles by avoiding commonly observed parasitic pathways, such as homodimerization or β-hydride elimination, thus leading to new knowledge in cross-electrophile reactions.

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